Manually update path_cache_storage

Is it possible to update the path_cache_storage (or path / local_storage) of a PublishedFile after it’s published? I’ve tried manually through the web:

image

And through the API:
shotgun.update("PublishedFile",24601, {"path_cache_storage" : {'code': 'primary', 'type': 'LocalStorage', 'id': 3}})

to no avail.

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